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https://itakigawa.github.io/ Exploring practices in machine learning and machine discovery for heterogeneous catalysis Ichi Takigawa Institute for Liberal Arts and Sciences, Kyoto University Institute for Chemical Reaction Design and Discovery, Hokkaido University RIKEN Center for Advanced Intelligence Project

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Share a viewpoint from the ML side (as I am an ML researcher, not a chemist) after >7 years struggling in heterogeneous catalyst design and discovery With great people in chemistry! Prof. Ken-ichi SHIMIZU Prof. Takashi TOYAO Prof. Satoru Takakusagi Prof. Zen Maeno Prof. Takashi Kamachi Keisuke Suzuki Shoma Kikuchi Shinya Mine Takumi Mukaiyama Motoshi Takao Yuan Jing Gang Wang Duotian Chen Kah Wei Ting Taichi Yamaguchi Koichi Matsushita S.M.A.H. Siddiki Prof. Koji Tsuda (U Tokyo) This talk

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Gas-phase reactions on solid-phase catalyst surface (Heterogeneous catalysis) Industrial Synthesis (e.g. Haber-Bosch), Automobile Exhaust Gas Purification, Methane Conversion, etc. https://en.wikipedia.org/wiki/Heterogeneous_catalysis Reactants (Gas) Catalysts (Solid) Nano-particle surface High Temperature, High Pressure Adsorption Diffusion Dissociation Recombination Desorption Heterogeneous catalysis

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Gas-phase reactions on solid-phase catalyst surface (Heterogeneous catalysis) Industrial Synthesis (e.g. Haber-Bosch), Automobile Exhaust Gas Purification, Methane Conversion, etc. https://en.wikipedia.org/wiki/Heterogeneous_catalysis Reactants (Gas) Catalysts (Solid) Nano-particle surface High Temperature, High Pressure Adsorption Diffusion Dissociation Recombination Desorption Involves devilishly complex too-many-factor processes. A solid surface shares its border with the external world. God made the bulk; the surface was invented by the devil —— Wolfgang Pauli Heterogeneous catalysis

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Accelerated discovery of multi-elemental reverse water-gas shift catalysts using extrapolative machine learning approach. https://doi.org/10.26434/chemrxiv-2022-695rj Our recent research: Results Our Target: Pt(3)/X1-X2-X3-X4-X5/TiO2 RWGS Calalyst

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Accelerated discovery of multi-elemental reverse water-gas shift catalysts using extrapolative machine learning approach. https://doi.org/10.26434/chemrxiv-2022-695rj • Discovered more than 100 catalysts better than the previously reported best catalyst. Our recent research: Results Our Target: Pt(3)/X1-X2-X3-X4-X5/TiO2 RWGS Calalyst

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Accelerated discovery of multi-elemental reverse water-gas shift catalysts using extrapolative machine learning approach. https://doi.org/10.26434/chemrxiv-2022-695rj • Discovered more than 100 catalysts better than the previously reported best catalyst. • 300 catalysts tested in total by 44 cycles of ML prediction + experiment Our recent research: Results Our Target: Pt(3)/X1-X2-X3-X4-X5/TiO2 RWGS Calalyst

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Accelerated discovery of multi-elemental reverse water-gas shift catalysts using extrapolative machine learning approach. https://doi.org/10.26434/chemrxiv-2022-695rj • Discovered more than 100 catalysts better than the previously reported best catalyst. • 300 catalysts tested in total by 44 cycles of ML prediction + experiment • The optimal catalyst Pt(3)/Rb(1)-Ba(1)- Mo(0.6)-Nb(0.2)/TiO2 was hardly predictable by human experts Our recent research: Results Our Target: Pt(3)/X1-X2-X3-X4-X5/TiO2 RWGS Calalyst

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Accelerated discovery of multi-elemental reverse water-gas shift catalysts using extrapolative machine learning approach. https://doi.org/10.26434/chemrxiv-2022-695rj • Discovered more than 100 catalysts better than the previously reported best catalyst. • 300 catalysts tested in total by 44 cycles of ML prediction + experiment • The optimal catalyst Pt(3)/Rb(1)-Ba(1)- Mo(0.6)-Nb(0.2)/TiO2 was hardly predictable by human experts • Notably, Nb was never used in training. Our recent research: Results Our Target: Pt(3)/X1-X2-X3-X4-X5/TiO2 RWGS Calalyst

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Decision tree ensembles (with UQ) i.e. histogram on data-dependent partitions • ExtraTrees regressor • Gradient Boosted Trees regressor + Abstracted (coarse grained) featurization of chemical compositions Input representations by elemental features e.g. “composition-based feature vector (CBFV)” Pt(3)/Ba(2)-Mo(1)-Tm(1)- Eu(0.5)-Dy(0.5)/TiO2 Pt(3)/Mo(1)-Ba(1)-Tb(1)- Ho(1)-Cs(0.5)/TiO2 Pt(3)/Rb(1)-Ba(1)- Mo(0.6)-Nb(0.2)/TiO2 Our recent research: Method

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Decision tree ensembles (with UQ) i.e. histogram on data-dependent partitions • ExtraTrees regressor • Gradient Boosted Trees regressor + Abstracted (coarse grained) featurization of chemical compositions Input representations by elemental features e.g. “composition-based feature vector (CBFV)” Pt(3)/Ba(2)-Mo(1)-Tm(1)- Eu(0.5)-Dy(0.5)/TiO2 Pt(3)/Mo(1)-Ba(1)-Tb(1)- Ho(1)-Cs(0.5)/TiO2 Pt(3)/Rb(1)-Ba(1)- Mo(0.6)-Nb(0.2)/TiO2 Very Conservative Prediction (Histogram) Very Radical Representation (Discard specific details) Our recent research: Method

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Decision tree ensembles (with UQ) i.e. histogram on data-dependent partitions • ExtraTrees regressor • Gradient Boosted Trees regressor + Abstracted (coarse grained) featurization of chemical compositions Input representations by elemental features e.g. “composition-based feature vector (CBFV)” Pt(3)/Ba(2)-Mo(1)-Tm(1)- Eu(0.5)-Dy(0.5)/TiO2 Pt(3)/Mo(1)-Ba(1)-Tb(1)- Ho(1)-Cs(0.5)/TiO2 Pt(3)/Rb(1)-Ba(1)- Mo(0.6)-Nb(0.2)/TiO2 This talk will hopefully explain why we go for such a standard method choice (even though I’m a ML researcher doing research also in GNNs and Transformers) Very Conservative Prediction (Histogram) Very Radical Representation (Discard specific details) Our recent research: Method

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At first I had an optimistic image of the unfamiliar field of "Materials Informatics"... (after I worked in machine learning for bioinformatics for 10 years) Step 1 Step 2 Step 3 We give all possible types of available data into ML ML becomes smarter than standard experts ML suggests more and more promising materials My prologue: Materials informatics?

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Three lessons learned as I experienced this illusion being shattered… Takeaways

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Three lessons learned as I experienced this illusion being shattered… 1. The goals of ML and ‘materials/chemical science’ are fundamentally different. What we need here is not ML but a much harder problem of ‘machine discovery.’ Takeaways

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Three lessons learned as I experienced this illusion being shattered… 1. The goals of ML and ‘materials/chemical science’ are fundamentally different. What we need here is not ML but a much harder problem of ‘machine discovery.’ 2. If we go for a hypothesis-free + off-the-shelf solution, exploration by decision tree ensembles, combined with UQ and abstracted (coarse grained) feature representations, will give a very strong baseline. Takeaways

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Three lessons learned as I experienced this illusion being shattered… 1. The goals of ML and ‘materials/chemical science’ are fundamentally different. What we need here is not ML but a much harder problem of ‘machine discovery.’ 2. If we go for a hypothesis-free + off-the-shelf solution, exploration by decision tree ensembles, combined with UQ and abstracted (coarse grained) feature representations, will give a very strong baseline. 3. If we want more than that, we can’t be hypothesis free. Any strategies to narrow down the scope as well as domain expertise really matters. Takeaways

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Get weight (g) & height (cm) Apple Orange Machine Learning converts data into predictions

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5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Apple Orange Machine Learning converts data into predictions

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5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Apple Orange Machine Learning converts data into predictions

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5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Apple Orange Machine Learning converts data into predictions

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5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Apple Orange Machine Learning converts data into predictions

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5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● 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● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Apple Orange Machine Learning converts data into predictions

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● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Apple Orange Machine Learning converts data into predictions

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Slide 25 text

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● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Apple Orange Machine Learning converts data into predictions

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● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ●● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● Get weight (g) & height (cm) Weight (g) Height (cm) Apple Orange Computer program for prediction Apple Orange Weight (g) Height (cm) Apple Orange Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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The computer program we got from training 5 6.25 7.5 8.75 10 90 112.5 135 157.5 180 ● ● ● ● ● ● ● ● ● ● Weight (g) Height (cm) Apple Orange Apple Orange weight (g) height (cm) This program can make prediction for different examples than the ones shown in training! Machine Learning converts data into predictions

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Synthesize a program (input-output function) just by giving input-output examples! Object Recognition “͋Γ͕ͱ͏” Speech Recognition J’aime la musique I love music Machine Translation Game Play Simple is better than Simple is better than complex Language Model ML = a new (lazy) way of computer programming!

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Synthesize a program (input-output function) just by giving input-output examples! Object Recognition “͋Γ͕ͱ͏” Speech Recognition J’aime la musique I love music Machine Translation Game Play N.B. This does not mean that we also “understood” the input-output relationship. Simple is better than Simple is better than complex Language Model ML = a new (lazy) way of computer programming!

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AlphaGo AlphaFold2 AlphaTensor ChatGPT Image Recognition Translation Image/Video Conversion “Deep Fake” Very powerful technology if we use it in the right place

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There are as many ML models as there are ways to draw the boundary… Decision Tree Random Forest GBDT Nearest Neighbor Logistic Regression SVM Gaussian Process Neural Network Data ML models are not unique even for the same dataset

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Every model just tries to fit a different type of functions to given data Classification Setup But all the inner workings are just function fitting to data

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Every model just tries to fit a different type of functions to given data y = 1 Classification Setup But all the inner workings are just function fitting to data

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Every model just tries to fit a different type of functions to given data y = 1 y = 0 Classification Setup But all the inner workings are just function fitting to data

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Every model just tries to fit a different type of functions to given data Random Forest Gaussian Process Logistic Regression P(class=red) Class probability y = 1 y = 0 Classification Setup But all the inner workings are just function fitting to data

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This fitting is done by optimally adjusting the model parameter values Random Forest Neural Network SVR Kernel Ridge p1 p2 p3 p4 Regression Setup By just tweaking numeric values for model parameters

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Three lessons learned as I experienced this illusion being shattered… 1. The goals of ML and ‘materials/chemical science’ are fundamentally different. What we need here is not ML but a much harder problem of ‘machine discovery’ 2. If we go for a hypothesis-free + off-the-shelf solution, exploration by decision tree ensembles, combined with UQ and abstracted (coarse grained) feature representations, will give a very strong baseline. 3. If we want more that that, we can’t be hypothesis free. Any strategies to narrow down the scope as well as domain expertise really matters. Takeaways

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To find "a material that is better than any existing materials today" or "a superior material that has never existed before. The goals are fundamentally di!erent.

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To find "a material that is better than any existing materials today" or "a superior material that has never existed before. To make a prediction for a given material on the basis of any similarities to the existing materials (i.e. the training data). The goals are fundamentally di!erent.

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To find "a material that is better than any existing materials today" or "a superior material that has never existed before. To make a prediction for a given material on the basis of any similarities to the existing materials (i.e. the training data). From a statistical point of view, this is the same as saying "I want outliers (exceptions).” The best known material is already a statistical outlier. The goals are fundamentally di!erent.

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Material’s performance 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 x AAAB93icbVDLSgNBEOyNrxhfUY9eFoPgKeyKr2PQi8cEzAOSJcxOepMhM7PLzKywhHyBVz17E69+jkf/xEmyBxMtaCiquunuChPOtPG8L6ewtr6xuVXcLu3s7u0flA+PWjpOFcUmjXmsOiHRyJnEpmGGYydRSETIsR2O72d++wmVZrF8NFmCgSBDySJGibFSI+uXK17Vm8P9S/ycVCBHvV/+7g1imgqUhnKiddf3EhNMiDKMcpyWeqnGhNAxGWLXUkkE6mAyP3Tqnlll4EaxsiWNO1d/T0yI0DoToe0UxIz0qjcT//O6qYlugwmTSWpQ0sWiKOWuid3Z1+6AKaSGZ5YQqpi91aUjogg1NpulLaGY2kz81QT+ktZF1b+uXjUuK7W7PJ0inMApnIMPN1CDB6hDEyggPMMLvDqZ8+a8Ox+L1oKTzxzDEpzPH5Ack50= y Material space Existing materials Known best I want material with larger anyway! 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 x AAAB93icbVDLSgNBEOyNrxhfUY9eFoPgKeyKr2PQi8cEzAOSJcxOepMhM7PLzKywhHyBVz17E69+jkf/xEmyBxMtaCiquunuChPOtPG8L6ewtr6xuVXcLu3s7u0flA+PWjpOFcUmjXmsOiHRyJnEpmGGYydRSETIsR2O72d++wmVZrF8NFmCgSBDySJGibFSI+uXK17Vm8P9S/ycVCBHvV/+7g1imgqUhnKiddf3EhNMiDKMcpyWeqnGhNAxGWLXUkkE6mAyP3Tqnlll4EaxsiWNO1d/T0yI0DoToe0UxIz0qjcT//O6qYlugwmTSWpQ0sWiKOWuid3Z1+6AKaSGZ5YQqpi91aUjogg1NpulLaGY2kz81QT+ktZF1b+uXjUuK7W7PJ0inMApnIMPN1CDB6hDEyggPMMLvDqZ8+a8Ox+L1oKTzxzDEpzPH5Ack50= y The setup is fundamentally di!erent from ML’s

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 x AAAB93icbVDLSgNBEOyNrxhfUY9eFoPgKeyKr2PQi8cEzAOSJcxOepMhM7PLzKywhHyBVz17E69+jkf/xEmyBxMtaCiquunuChPOtPG8L6ewtr6xuVXcLu3s7u0flA+PWjpOFcUmjXmsOiHRyJnEpmGGYydRSETIsR2O72d++wmVZrF8NFmCgSBDySJGibFSI+uXK17Vm8P9S/ycVCBHvV/+7g1imgqUhnKiddf3EhNMiDKMcpyWeqnGhNAxGWLXUkkE6mAyP3Tqnlll4EaxsiWNO1d/T0yI0DoToe0UxIz0qjcT//O6qYlugwmTSWpQ0sWiKOWuid3Z1+6AKaSGZ5YQqpi91aUjogg1NpulLaGY2kz81QT+ktZF1b+uXjUuK7W7PJ0inMApnIMPN1CDB6hDEyggPMMLvDqZ8+a8Ox+L1oKTzxzDEpzPH5Ack50= y Material’s performance Material space ML predicted values cut through the middle of the given training samples. An inconvenient truth: ML is useless for this purpose

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 x AAAB93icbVDLSgNBEOyNrxhfUY9eFoPgKeyKr2PQi8cEzAOSJcxOepMhM7PLzKywhHyBVz17E69+jkf/xEmyBxMtaCiquunuChPOtPG8L6ewtr6xuVXcLu3s7u0flA+PWjpOFcUmjXmsOiHRyJnEpmGGYydRSETIsR2O72d++wmVZrF8NFmCgSBDySJGibFSI+uXK17Vm8P9S/ycVCBHvV/+7g1imgqUhnKiddf3EhNMiDKMcpyWeqnGhNAxGWLXUkkE6mAyP3Tqnlll4EaxsiWNO1d/T0yI0DoToe0UxIz0qjcT//O6qYlugwmTSWpQ0sWiKOWuid3Z1+6AKaSGZ5YQqpi91aUjogg1NpulLaGY2kz81QT+ktZF1b+uXjUuK7W7PJ0inMApnIMPN1CDB6hDEyggPMMLvDqZ8+a8Ox+L1oKTzxzDEpzPH5Ack50= y In conclusion, ML can’t predict better material than ones in the training data Material’s performance Material space ML predicted values cut through the middle of the given training samples. i.e. they take mediocre values between the best and worst values in the training data. An inconvenient truth: ML is useless for this purpose

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• This is not a bug, it’s a feature! It’s not a bug, it’s a feature

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• This is not a bug, it’s a feature! If we already have sufficient data, experts would already identify promising materials and there is no need to use ML predictions. • Furthermore, “Let’s try ML” situations usually imply the paucity of data. It’s not a bug, it’s a feature

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• This is not a bug, it’s a feature! • In such a situation, it is extremely difficult to accurately evaluate the ML predictions since it means that we don’t have enough data for testing either. If we already have sufficient data, experts would already identify promising materials and there is no need to use ML predictions. • Furthermore, “Let’s try ML” situations usually imply the paucity of data. It’s not a bug, it’s a feature

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• This is not a bug, it’s a feature! • In such a situation, it is extremely difficult to accurately evaluate the ML predictions since it means that we don’t have enough data for testing either. If we already have sufficient data, experts would already identify promising materials and there is no need to use ML predictions. • Furthermore, “Let’s try ML” situations usually imply the paucity of data. It is a matter of course for ML to be able to predict the training examples. So we need to ensure if ML can predict other examples than the training ones. However, test data means everything but the training examples… It’s not a bug, it’s a feature

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For discovery, accurate prediction for the entire input space is expected because we are interested in any possible materials! (no probability things here) AAAChHichVHLTsJAFD3UF+ID1I2JGyLBuDBkUHzEhSG6cclDHgkS0tYBG0rbtIUEiT+gW40LV5q4MH6AH+DGH3DBJxiXmLhx4aU0MUrE20znzJl77pyZKxmqYtmMtT3C0PDI6Jh33DcxOTXtD8zMZi29bso8I+uqbuYl0eKqovGMrdgqzxsmF2uSynNSda+7n2tw01J07cBuGrxYEyuaUlZk0SYq2SwFQizCnAj2g6gLQnAjoQcecYgj6JBRRw0cGmzCKkRY9BUQBYNBXBEt4kxCirPPcQofaeuUxSlDJLZK/wqtCi6r0bpb03LUMp2i0jBJGUSYvbB71mHP7IG9ss8/a7WcGl0vTZqlnpYbJf/ZfPrjX1WNZhvH36qBnm2UseV4Vci74TDdW8g9fePkqpPeToVbS+yWvZH/G9ZmT3QDrfEu3yV56nqAH4m80ItRg6K/29EPsquR6EYkloyF4rtuq7xYwCKWqR+biGMfCWSoPsc5LnApjAorwpqw3ksVPK5mDj9C2PkC2GOP+Q== y 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 x1 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 x2 Test data Materials/Chemical Sciences The training and test data also fundamentally di!er

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For discovery, accurate prediction for the entire input space is expected because we are interested in any possible materials! (no probability things here) 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 y 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 x1 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 x2 Test data Materials/Chemical Sciences Training samples should cover the entire input space. Training data 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 y 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 x1 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 x2 With considering Fisher’s three principles for DoE. Replication, Randomization, Local Control (Blocking) The training and test data also fundamentally di!er

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For discovery, accurate prediction for the entire input space is expected because we are interested in any possible materials! 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 x2 Test data Materials/Chemical Sciences Machine Learning Out-of-sample area ignored 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 y 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 x2 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 x2 Test data Training data Both samples follow the same distribution Training samples should cover the entire input space. Training data 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 y 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 x1 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 x2 With considering Fisher’s three principles for DoE. Replication, Randomization, Local Control (Blocking) The training and test data also fundamentally di!er

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We should recognize this problem as a quite different problem from standard ML! “Machine Discovery” Problem

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We should recognize this problem as a quite different problem from standard ML! Herbert A. Simon • Simon, Machine Discovery. (1997) • Langley, Simon, Bradshaw, Zytkow, Scientific Discovery: Computational Explorations of the Creative Process (1987). • Arikawa, Our Studies on Machine Learning and Machine Discovery. (1996) • Arikawa et al, The Discovery Science Project (2000). Setsuo Arikawa Won Nobel Prize & Turing Award It is way harder than ML, and requires systematic study on whether any ‘scientific discovery’ can be rationalized by using “hard” sciences as a compelling testbed. Indeed now is the best time to revisit this theme with modern methods and data. Human and machine discovery are gradual problem-solving processes of searching large problem spaces for incompletely defined goal objects. (Simon) “Machine Discovery” Problem

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Three lessons learned as I experienced this illusion being shattered… 1. The goals of ML and ‘materials/chemical science’ are fundamentally different. What we need here is not ML but a much harder problem of ‘machine discovery’ 2. If we go for a hypothesis-free + off-the-shelf solution, exploration by decision tree ensembles, combined with UQ and abstracted (coarse grained) feature representations, will give a very strong baseline. 3. If we want more that that, we can’t be hypothesis free. Any strategies to narrow down the scope as well as domain expertise really matters. Takeaways

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Inconvenient mathematical truths (Curse of dimensionality) 1. The number of samples required to ensure the accurate prediction for the entire input space (uniform approximation) is necessarily exponential in the dimension. If we take 5 levels for each variable, we need 52 = 25 for 2 variables; we need 510 ≈ 10 millions for just 10 variables. Approx for the entire input space is practically impossible

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Inconvenient mathematical truths (Curse of dimensionality) 1. The number of samples required to ensure the accurate prediction for the entire input space (uniform approximation) is necessarily exponential in the dimension. If we take 5 levels for each variable, we need 52 = 25 for 2 variables; we need 510 ≈ 10 millions for just 10 variables. 2. The probability that a new sample falls in training set’s convex hull is almost zero for a high-dimensional (>100) space. Interpolation almost surely never happens, and “Learning in high dimension always amounts to extrapolation”. (Balestriero, Pesenti, LeCun, 2021; arXiv:2110.09485) Approx for the entire input space is practically impossible

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= + + + + + i.e. Histogram rules on data-dependent partitions (piecewise constant) (piecewise constant) • Make prediction by a histogram rule, i.e. the average of subset of training samples even for the out-of-sample area • It’s a histogram and unintentional interpolation just by ungrounded inductive biases never happens even in a high- dimensional space. Decision tree ensembles: Local-averaging estimators

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= + + + + + i.e. Histogram rules on data-dependent partitions (piecewise constant) (piecewise constant) • Make prediction by a histogram rule, i.e. the average of subset of training samples even for the out-of-sample area • It’s a histogram and unintentional interpolation just by ungrounded inductive biases never happens even in a high- dimensional space. Decision tree ensembles: Local-averaging estimators

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= + + + + + Average of samples’ y in the area i.e. Histogram rules on data-dependent partitions (piecewise constant) (piecewise constant) • Make prediction by a histogram rule, i.e. the average of subset of training samples even for the out-of-sample area • It’s a histogram and unintentional interpolation just by ungrounded inductive biases never happens even in a high- dimensional space. Decision tree ensembles: Local-averaging estimators

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= + + + + + Average of samples’ y in the area i.e. Histogram rules on data-dependent partitions (piecewise constant) (piecewise constant) • Make prediction by a histogram rule, i.e. the average of subset of training samples even for the out-of-sample area • It’s a histogram and unintentional interpolation just by ungrounded inductive biases never happens even in a high- dimensional space. Decision tree ensembles: Local-averaging estimators

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KernelRidge(kernel='rbf', alpha=0.05, gamma=0.1) KernelRidge(kernel='rbf', alpha=1e-4, gamma=0.1) KernelRidge(kernel='rbf', alpha=1e-4, gamma=2.0) Evidence-based behavior for out-of-sample area For out-of-sample area, we cannot say anything confident without any assumptions by inductive biases (continuity)

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KernelRidge(kernel='rbf', alpha=0.05, gamma=0.1) KernelRidge(kernel='rbf', alpha=1e-4, gamma=0.1) KernelRidge(kernel='rbf', alpha=1e-4, gamma=2.0) Evidence-based behavior for out-of-sample area For out-of-sample area, we cannot say anything confident without any assumptions by inductive biases (continuity) But this can be not necessarily continuous (selectivity cliffs, activity cliffs, etc)

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KernelRidge(kernel='rbf', alpha=0.05, gamma=0.1) KernelRidge(kernel='rbf', alpha=1e-4, gamma=0.1) KernelRidge(kernel='rbf', alpha=1e-4, gamma=2.0) Evidence-based behavior for out-of-sample area For out-of-sample area, we cannot say anything confident without any assumptions by inductive biases (continuity) But this can be not necessarily continuous (selectivity cliffs, activity cliffs, etc) ExtraTreesRegressor(n_estimators=50) DecisionTreeRegressor() conservative and safer prediction at least, grounded by some given data

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PolyReg(1) RMSE 0.299 PolyReg(3) RMSE 0.28 PolyReg(5) RMSE 0.225 PolyReg(7) RMSE 0.113 PolyReg(10) RMSE 0.0189 PolyReg(15) RMSE 0.00737 PolyReg(20) RMSE 0.000 PolyReg(30) RMSE 0.000 ExtraTrees (no bootstrap) RMSE 0.000 ExtraTrees (bootstrap) RMSE 0.0121 Random Forest RMSE 0.012 Light GBM RMSE 0.0508 95% PI 95% PI 95% PI 95% PI Problematic overfitting by polynomial regression of order k Clearly overfitted but harmless (still informative) Adaptability for non-smooth changes (Benign overfitting)

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Geurts, Ernst, Wehenkel, Extremely randomized trees. Mach Learn 63, 3–42 (2006). https://doi.org/10.1007/s10994-006-6226-1 ExtraTreesRegressor(n_estimators=10) RandomForestRegressor(n_estimators=10) Pseudo-continuous interpolation of ExtraTrees

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Decision tree ensembles (with UQ) i.e. histogram on data-dependent partitions + Abstracted (coarse grained) featurization of chemical compositions Pt(3)/Ba(2)-Mo(1)-Tm(1)- Eu(0.5)-Dy(0.5)/TiO2 Pt(3)/Mo(1)-Ba(1)-Tb(1)- Ho(1)-Cs(0.5)/TiO2 Pt(3)/Rb(1)-Ba(1)- Mo(0.6)-Nb(0.2)/TiO2 Very Conservative Prediction Very Radical Representation • Evidence-based behavior for out-of- sample area • Adaptability for non-smooth changes • avoid fragmented memorization • compensate for elemental sparsity and data paucity Our recent research: Method

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Three lessons learned as I experienced this illusion being shattered… 1. The goals of ML and ‘materials/chemical science’ are fundamentally different. What we need here is not ML but a much harder problem of ‘machine discovery’ 2. If we go for a hypothesis-free + off-the-shelf solution, exploration by decision tree ensembles, combined with UQ and abstracted (coarse grained) feature representations, will give a very strong baseline. 3. If we want more that that, we can’t be hypothesis free. Any strategies to narrow down the scope as well as domain expertise really matters. Takeaways

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Can ML contribute to scientific discovery/understanding? I assume that ML-based exploration like ours is used, calibrated, and carefully monitored by human experts. I am skeptical so far about whether scientific discovery can be fully automated by AI. º What kinds of elemental features are used…? What level of coarse graining is effective…? :

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Can ML contribute to scientific discovery/understanding? I assume that ML-based exploration like ours is used, calibrated, and carefully monitored by human experts. I am skeptical so far about whether scientific discovery can be fully automated by AI. • In the first place, the majority of scientific research, particularly experimental science, is still largely empirical, and much is irrationally left to luck and inertia. º What kinds of elemental features are used…? What level of coarse graining is effective…? :

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Can ML contribute to scientific discovery/understanding? I assume that ML-based exploration like ours is used, calibrated, and carefully monitored by human experts. I am skeptical so far about whether scientific discovery can be fully automated by AI. • In the first place, the majority of scientific research, particularly experimental science, is still largely empirical, and much is irrationally left to luck and inertia. • ML-based exploration is just a glorified version of empirical exploration, and exhibits different types of “bounded rationality (Herb Simon again!)” as we are bounded by our own “cognitive limits.” º What kinds of elemental features are used…? What level of coarse graining is effective…? :

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We cannot be hypothesis free when we want causality. Science requires causal understanding

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We cannot be hypothesis free when we want causality. • “Causal analysis is emphatically not just about data; in causal analysis we must incorporate some understanding of the process that produces the data, and then we get something that was not in the data to begin with.” Science requires causal understanding

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We cannot be hypothesis free when we want causality. • “Causal analysis is emphatically not just about data; in causal analysis we must incorporate some understanding of the process that produces the data, and then we get something that was not in the data to begin with.” • “Unlike correlation and most of the other tools of mainstream statistics, causal analysis requires the user to make a subjective commitment.” Science requires causal understanding

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We cannot be hypothesis free when we want causality. • “Causal analysis is emphatically not just about data; in causal analysis we must incorporate some understanding of the process that produces the data, and then we get something that was not in the data to begin with.” • “Unlike correlation and most of the other tools of mainstream statistics, causal analysis requires the user to make a subjective commitment.” Science requires causal understanding For causal understanding, data is not everything. We need something else that doesn’t come from the data themselves.

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Science is built up with facts, as a house is with stones. But a collection of facts is no more a science than a heap of stones is a house. Henri Poincaré “Science and Hypothesis” ML gives prediction; We want discovery/understanding

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• “Theory-driven models can be wrong. But data-driven models cannot be wrong or right. Data-driven are not trying to describe an underlying reality.” (David Hand) Science is built up with facts, as a house is with stones. But a collection of facts is no more a science than a heap of stones is a house. Henri Poincaré “Science and Hypothesis” ML gives prediction; We want discovery/understanding

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• “Theory-driven models can be wrong. But data-driven models cannot be wrong or right. Data-driven are not trying to describe an underlying reality.” (David Hand) • “The goal of finding models that are predictively accurate differs from the goal of finding models that are true.” Statistical Learning from a regression perspective. Science is built up with facts, as a house is with stones. But a collection of facts is no more a science than a heap of stones is a house. Henri Poincaré “Science and Hypothesis” ML gives prediction; We want discovery/understanding

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• “Theory-driven models can be wrong. But data-driven models cannot be wrong or right. Data-driven are not trying to describe an underlying reality.” (David Hand) • “The goal of finding models that are predictively accurate differs from the goal of finding models that are true.” Statistical Learning from a regression perspective. Science is built up with facts, as a house is with stones. But a collection of facts is no more a science than a heap of stones is a house. Henri Poincaré “Science and Hypothesis” ML gives prediction; We want discovery/understanding If we seek not prediction but (scientific) understanding, we basically cannot remain hypothesis-free because “understanding” is the problem of human recognition.

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e.g. The universal approximation theorem says that neural networks can approximate any function. Giving Up on ML’s Versatility Modern ML models have the virtue of being able to represent any function just by changing parameter values. “Blackbox” vs. “Hypothesis-free”

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e.g. The universal approximation theorem says that neural networks can approximate any function. Giving Up on ML’s Versatility Modern ML models have the virtue of being able to represent any function just by changing parameter values. “Blackbox” vs. “Hypothesis-free”

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e.g. The universal approximation theorem says that neural networks can approximate any function. Giving Up on ML’s Versatility Modern ML models have the virtue of being able to represent any function just by changing parameter values. “Blackbox” vs. “Hypothesis-free” • However, when used in the natural sciences, this virtue leads to scientifically invalid predictions just by "spurious correlations” in the given finite data…

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e.g. The universal approximation theorem says that neural networks can approximate any function. Giving Up on ML’s Versatility Modern ML models have the virtue of being able to represent any function just by changing parameter values. “Blackbox” vs. “Hypothesis-free” • However, when used in the natural sciences, this virtue leads to scientifically invalid predictions just by "spurious correlations” in the given finite data… • It is not good to be able to "represent any function," but it is better to restrict the model so that “it cannot represent scientifically invalid functions by design.”

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https://doi.org/10.1038/s42254-021-00314-5 • Theory • Simulation Machine Learning Physics Data Sim2Real Geometric ML Data Assimilation Simulation with Prediction • ML × Simulation • ML × Theoretical Chemistry/Physics • ML × Logic & Symbol Manipulations Fusion between rationalism & empiricism (deduction & induction) Path to Machine Discovery: 1st step is physics-informed?

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Three lessons learned as I experienced this illusion being shattered… 1. The goals of ML and ‘materials/chemical science’ are fundamentally different. What we need here is not ML but a much harder problem of ‘machine discovery’ 2. If we go for a hypothesis-free + off-the-shelf solution, exploration by decision tree ensembles, combined with UQ and abstracted (coarse grained) feature representations, will give a very strong baseline. 3. If we want more that that, we can’t be hypothesis free. Any strategies to narrow down the scope as well as domain expertise really matters. PDF of this slide: https://itakigawa.page.link/acs2023spring Summary